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Full text of "The velocity and ratio e/m for the primary and secondary [Beta] rays of radium .."

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THE VEIOCTTY \'''V '^'VTIO _e_ FOR TtlE 

m 

PRI"ARY MW ?ECONr/VRY 3 RAYS 
OF •R'.rTil''. 



BY 



S.J. ALLEN. 



DISSERTATION 
SUBVITTED TO THE BOA.RD OF UNIVERSITY STUTIES 

OF THE JOHNS HOPKINS UNIVERSITY 
IN CO'TOR"ITY WITH THE REOUIRE"ENTS FOR THE 

TEGREE OF DOCTOR OF PHILOSOPHY. 



BALTIMORE 
1906. 



r^iroL 






THE YEIOCITY \'ir RATIO _^ FOR THE' 
PRI^'ARY AND SECONDARY P RAYS 

OF R'\ri'.r". 



3Y 
S.J. ALl.KN. 



BIOGRAPHY. 



Sa"i.uel James "aclr.toyh "lien was born at "aitland, 
"Jova rcotia on October 5th, 1877. Hia earlier educatjon 
was r.ainod in the public and private schools, and in the 
Halifax High rchool from whicn ha rraduated in 189 5. In 
IB^G he entered the depirtnent of Electrical Engineering 
at "c^ill 'Jni versi tjr , "ortreal, Canada, and graduated 
witi tne de-^ree of B . r- c . in 1.^00. On rTaduation ho .vas 
appointed demonstrator in the Engine eri nrr laboratories, 
where he ras also enraged in research vTork on "The Plow of 
"Vater throurh Pipes 'ind Hends", for 'Yni ch in ijOl he vas 
awarded the derroe of ''.."vc. He was then appointed demon- 
strator in the '^hy;-ical laboratory at the same university, 
w:iere he re"iained for the next two years engap^ed durinr 
a great part of the time in researches on "The Radioactivity 
of the'i.t mo sphere", both in conns ct ion with Professor 
Rutherford and alone. The result of these Inve sti -ation s 
has been published in various articles in the Phil, "a?., 
Phys. Review, Phys. Zeit., and other journals. 

In 1903 he entered the graduate department of Physics 
in the Johns Hopkins University , obtaining the Fellowship 
in ^hysics for the rear 1903-01:. Turing his course at 
this Hniversit" n p has st'aried under Professor Ames, Pro- 
fessor IVood, Professor Jones and Professor "orley- his 



principal subject being Physicn, first subordinate "Physi- 
cal Che'^.i^tr^' and srecond subordinate ''at henati cs . 

''r. Mien is a "ie"iber of the Canadian ^ocietv of 
Civil Engineers and the ^r.srican Phvr;.ical "ociety. 



INTRODUCTION. 



The reasons which led the author to : n v e s t i "■ a t e this 
subject ought first to bo briefly stated. V/n.ile trying 
to denonstrate experinmntal ly the iiagnetic and electro- 
static devia+jon of the 3 rays from radiun, by means of 
the electrical '-.etnod, I was surprised to find that no 
appreciable electrostatic deflection could bo obtained 
by tne methods ax first used, and that moreover tne mag- 
netic deflection observed v/ a s rn u c n less than '^ e i.v o u 1 d 
be led to pxpect frora the results of ether e xper iraenter s • 
Considerinp: the great importance of this subject, affording 
as it does the only metnod ffn nave for testing the be- 
haviour of the electron at speeds approacning that of 
light, it was deeded advisable to nuke a thorough inves- 
tir,at:'on, and to find out, if possible, \\rherein lay 
the difficulties, and the non-success of zae early 
experiments. 

Before describing ny own experiments it will be 

of interest to y'ive a brief resume of the \^/ork done by 

previous investigators on this subject, and the conclu- 

1 
sions reached by thera. Becquerel v/as the first to state 

1 . C". V. " 13 O", ' 1 9 f'.". 



that the P rays fron rad'^un vrere deflected in an elec- 
trojjtatic field; wad by "usas <r i nf; this deflection, 
and knowing frcn earlier experiinents the deflection of 
the sane rays in a magnetic field, he was able to cal- 
culate their velocity, and the ratio ^. e being the 
charge in ele ctro otati c C.G.S. units, und 21 tae mass 
expressed in grammes. 

His experi.Tiental method aight be briefly described 
as follows. A. pencil of 3 rays v/as allo^sd to pass 
upward bet\-reon two parallel brass plates, and to fall 
upon a photogra[>hic film, placed horizontally above 
t>.em. The plates were insulated from one another, and 
maintained at a high difference of potential by means of 
an electrostatic machine. A tnin slieet of mica v/as 
placed vertically in tie path of the rays, so as to 
cut it into two nalves. ihe image on the photographic 
film would thus l-e divided into two parts by a fins 
line in the ce-'tre. If now on ttie application of an 
electrostatic field the rays are bent, then there 
ought to appear on the image a shadow, the widtli of 
v/i-:ich ./ould co-^respr,nd to the least deviable ray. 

Becquerel observed such a shadow, and measuring 
the wid+ (f it, ■ind knowing from other e x;^er iment s 



the value of the t". a r r. e t i c deflection, hu calculated 

10 

tne velccitv of the P particle to be about 1.6 x 30 

7 

ens. per sec., and the ratio je_ :i s 1 x 1 . T li i s 

fn 

experi.r. ent of Becquerel was "■iude in air at atnospheric 
pressure, and for this reaeon no very accurate esti-^ate 
of tiie true sl:ctric field betv/een the plates could 
be -".ads, sinue t::e ionization cauted by the B rays v/ould 
to a great extent disturb the potential gradient. 
The results of iiecquerel can therefore be only con- 
sidered as ap'iro xi nat e . 

1 
The "lethod used by Kaufmann to obtain the velocities 

of the ,3 rays was entire I37 different and .vas based on 
the principle of crossed spectra. The hetero2;eneous 
pencil of rays from a s'lall speck of radium passed 
upv/ard ijetv^een two brass plates, through a small hole 
in a netal diaphragm, placed !icr i zontal] j' above the 
plates, and then fell normally upon a photographic 
plate, wrapped in a thin envelope of aluminium. The 
brassplates were insulated froxn one another and could 
be kept charged to a high difference of potential by 
.Tieans of a battery of small lead ac curriul^.tor s . The 
whole apparatus v/as enclosed inside a glass vessel from 
which the air could be exhausted. A -na:^netic fisld was 
1. Nachr. d. (".esT d . V/'ei's'ii" m" G t't'. ", ~ 1 9 iT [ 



applied parallel tc the electrostatic and an exposure 
given for a certain time; tile c;irecti.on of the electrc 
static field was then reversed, -intl i further expos- 
ure of the fja-ne time as before piiven, the direct:ion 
of the magnetic field beinr tho same in both cases. 
'iVhen trie pls-te •vas developed there a-^'Oeared on it 
t'vo curveri lines, snovving that the (3 particles had 
been deflected by both the m.a,7netic and electrostatic 
fields. By measuring the deflections obs8""ed, the 
value of the velocity, and ^ for each rav could be 

calculated. lie found that the velocities varied from 

10 lO 

2.36 xlO to 2.85 xlO , and the value of €^ from 

7 7 )n 

1.31 X IC to .63 X 10 . Assuming; that the charfre is 

constant, these results showed that the mass of the 
electron apparently increased as the velocity of 
light was approached. 

A theory nas been developed by Thomsonjand elab- 
orated b^r Heaviside, Abraham, and o t her s - '.'/hereby the 
mass of the elsctrojj is considered as entirely elec- 
trical in its nature, and increases with the speed 
of the electron, reachin,?^ at the velocity of lifht 
an infinite value. The late values of ^ obtained 

m 

by Kaufmann agreed very well with those as calcu- 
lated from the formulae of Abraham. I shall discuss 



■t 



these results later on in this paper. 



ELECTRICAL EXPERI'^ENTS . 
The electrical 'nethod, whenever prtictical, is 
in some respects to be preferred to the photographic, 
in as nuch as many readings can be •'ade and confirT.ed 
in the same ti'^e tnat it takes to 'nake -i sinf;le expos- 
ure by the latter. In my first experir.ents a sensi- 
tive Dolezalek electror^eter fras used, but it *as 
found a I" Oft i r^'.no ss :1 bl e to shield this and the 
connecting v/ires fron electrostatic influences 
sufficiently to obtain accurate readings. It was 
therefore replaced by a sensitive t^old leaf elec- 
troscope, which could be shielded very ea.':il3'' from 
the effects of the hif^h potentials uced. 
Expe r i ne nt I . 

The fi'-st experi^nent was tried in air at atnos- 
p.heric nressure, and the general ar'"ar<^e'':ent is shown 
sketched in Fig. T. Two zinc plates 18 c's. long 
were attached to insulating uprights •'*. and B, which 
kept then in a vertical position about 9 r;"is. apart. 
At the bottom of the plates was placed a block of lead 
containing some radium bromide, covered ?/ith a thin 
sheet cf .mica, vrr.ich allowed the 8 rays to pass through 




^ Earth. 



a I 



Earth 



A 



B 



Radium 



VI 0,1- 



'jtp.out 'luch abse?-T.t3on . The radium msls r,o arranged 
that it' extrene edre -vay i'^ a vertical line twith 
tne plate b, thus causing the rays to rraze the plite 
b, but iJJowing the-! to fall fulD upon the plate a. 

Over the top of the plates 'i^as sus^'ended the elec- 
troscope, the details of >.vh3ch are shown in the 
fjc'uro. The rod c containing tne fold leaf was 
insulated from the case by -^eans of a bead of sul- 
phur e. The syste-^ was charged to a potential of a 
few hundred volts by means of the rod f, wnich could 
be turned so as to touch the rod holding the gold 
leaf. At other tJ-^-es it was con-iected to the case, 
which was eartned. Tne bottom of the electroscope 
had a thin aluminium windov»r throuph whJch the rays 
could pass. The time which the cold leaf took to 
fall thT-cufh a fixed distance on the cross hair of tne 
telescope was taken as a measure of the ionization, 
'^art of this ionization was due to tne 8 and secon- 
dary ravs, and part to the Y radisAtions, and these 
could be di sti nFuisned from one finother by absorption 
tests. Of tie total about 60-^ was due to tne V" and 
the remainder to 3 and cecondarv ra-"s. 

If noiv 1-iie plate a i ;^ charped positively, then 
the 3 ravs snould be deflected away from the plate 



\. 



b, unci a decrease of tne ionization observed. Triis 
cecrease v/ould be a "teasure of the deflection of the 
rays since no fresh rays could be bent in to take the 
place of t-iose bent away . If the. rays travel -it dif- 
ferent velocities, then tnis deflection ./i-uid be only 
an averat^.e value, but by absorbing tne ones of lov^rer 
veJocity one ourht tu be able to obtain tne deflection 
of the hirn velocity rays very approximately. 

The plates were "^aintarnad at a difierence of 
potential by connecting them to a battery of small lead 
accumulators, from v/hich a max.imum potential of 5000 
volts could be obtained. In tne later experiments tne 
number of colls rfas increased, so that a potential 
difference of about 9000 volts was available. 

"fhen a difference of potential of 3000 was applied 
to the plates no appreciable decrease of the ioniza- 
tion in the electroscope could be observed. The rays 
were completely deflected by means of a mapnetic field, 
but the value of HP., H being the strength of the mag- 
netic field, and r tie raidus of curvature of tne 
deflected rays, as calculated from this deflection was 
over five times what it snould have i;een calculated 
from t n e o r y . 



The expression for the deflection of the ruy in 
a uniform electrostatic field iej- 

where 5 represents the uaflHct'on, d the distance trav- 
elled by the ray in ^he field, h the distunce from 
the top of the plates to the electroscope, e the 

m 

ratio of charge to nass of the electron, X the 

strength of the electric field, and V the velocity 

of the electron. In this experiment d = 18 c"-.s., h 

11 
= 7 ens. and K = 5 x 10 e • m . units. 

If we as'^ume for V, and ^_, the extre"ie vt-ilues 

m 10 

found 1-jy Kaufrnann, viz., 2.8j x 10 cms. per sec, 

7 
f\nd .63 X 10 , the calculated value of the electro- 
static deflection for th<t hifhest velocity rays 
amounts to about 11 mm. v/hi(;h should have been 
observed since the yidth of tne window of tne elec- 
troscope vas only 15 mns. 

This failure to observe the electrostatic de- 
flection could not at first be satisfactorily ex- 
plained, and it >vas only after a number of expe^ i^^ent s 
by different methods were .r.ade that the true expla- 
nation vas reached. I shall discuss this point later on 



In this expsriaent , as in all otners made in air at 
atmospheric pressure, .ve have no ver;,^ definite knov/1- 
edhe of cue aniformity of the electric field bet.veen 
the plates, and for this reason all the remaining 
expsriments v/ere carried out in a vacuua. In tais 
case the plates can be placed closer to?^,etaer, and a 
auch higher potential applied oetveon the m v/ithcut 
a dischar.tye taking place, tne field between tne plates 
beinp; r-ractically uniform. 
Experim ent II « 

In fig. TI is sketched tne general arrange- 
ment of tnis experiment. Two zinc plates, a and b, 6 c -g 
long are insulated from one another, and kept a dis- 
tance apart of 3.9 mms. by means of ebonite side pieces. 
Beneath- tiie plates are fastened tiVo ebonite blocks, 
forming betttecn tnem a slit of about 1 mm .vidth, tnrough 
v/hich pass the rays from the radium contained in a cap- 
sule placed below. The capsule is covered vith a thin 
sheet of mica, and sealed so that no emanation from tne 
radium can escape into the surrounding vessel. 

Tnis apparatus was then enclosed in;:ide a glass 
vessel k from Afhich tne air could be exhausted to a 
high vacuum. The top of the vessel was closed by means 



Elechoscope 



/ 



C 



D 



'»*>n->"3- 




'■'-^--'■'-1 




Radium 



F.gl- 



of !i brass cap B, ^vaici .lud an opening cut tnrouph it, 
and covered.vnth a very thin sheet of zir.c. T//o //ires 
sealed t ii r o u g h the glass were connected to the two 
plates, rind served to charj^e them to any desired po- 
tential difference- 
On top of the brass cap .vsre placed t'//o parallel 
brass blocks, 3 cms. long and at a distance apart of 
1 cm., v/hich supported the elnctroscope. 

The rays fro"i the radium passed upward in a 
diverging bean, through the thin saeet of zinc,a'"-d 
into the electroscope. When the vessel was exh-tusted 
to a high vacuum the plates maintained a potential 
difference of 5000 volts without a discharre; in 
this case we can assume that the electric field between 
the plates is uniform. When this voltage, which corre- 
sponds, to an electric field of about 17000 volts per cm,, 
v/as applied there .vas a decrease of aoout 10-15 per cent 
in tne ionization due to 3 rays. The rays >vhich reach 
tae electroscope will consist in a larf;;e part of 
those of r.edium and high velocities, sicca the low 
velocity rays are nostly absorbed in the zinc plate. 
If v/e calculate as before tne deflection which might be 
looked for we find it to be about 3.2 m'-.s. for the 
highest velocity rays, and since the distance betAfeen 



10 



the plates at t'ne electroscope is only 10 m-is^ tr.is 
would a"iount to over 80^= conplete deflfctnon. Those rays 
of lever velocity would be coapletely def ected. Haen 
the apparatus was pl±ced in a nupnetic field the rays 
could be completely deflected, though tne apparent 
value of HR obtained whs over three ti"iss what it might 
be looked for. 

There v/ a s a slight possibility that 3 o m e of the 
emanation might have escaped into the vessel, in which 
case the true effect would be to sone extent masked by 
the rays coning from the emanation. In order to prevent 
this possibili-py anotner ar '-ange-ent was devised //here 
the radium was kept entirely outside the vessel contain- 
ing the charged plates. 
Exper i me nt II I . 

The experi lental arrnngement is shown in fig. IV. 
A series of zinc plates, a , a , a , etc., IS in. number 
were arranged parallel to one another, being insulated 
and kept arart from one another by means of ebcntie side 
strips. This a^range-^ent v/as enclosed int-ide a glass 
vessel A, which had the wall? blown out in thin bulbs 
immediately above and below the system of parallel plates^ 



Electroscope 




Radium 



FiqW 



11 



Alternate platPB .irere connected toretr.er and tc one 
electrode, tne re"ia?.ninp plates bein?^ joined to the 
other electrode. Tne lo-rta of the pl&tes .vas t c-,s., 
and the dist'^nce apart 1 mm.. The radium was placed 
beneath the plates, and the electroscope above. By this 
arrar.genent a :^.uch greater a'lount off? rays could get 
into the electroscope than in the previous e xper 5 iisnt a , 
and also a large electric field cculd be prccuced 
between the plates. A s all deflection of the rays 
should be rBadily detected in tne electroscope. The 
radium •ras placed about 4 c^^b. fro-n the botto'Ti of the 
plates, so that the increase due to rayb being bent so 
as tc ente'- the electroscope could not be great enough 
to offset the dec-ease due to rays bent away and absorbed. 

'Hhen s. difference of potential of 5000 volts ^vas ap- 
plied to the pl:ttes no very appreciable deflection cculd 
be observed. T::e magnetic deflection was also consid- 
erably less than one r-iight expect froir. theory. The 
total thickness of the glass walls wc<ld have about the 
same absorbing power as tne sheet of zinc in the previous 
experiment . 

The results of these experiments frere at first very 
perplexing, and no very satisfactory explanation could 



12. 



be reac.ied. One was loath tc concludo that tlie 3 rays 
v/ere not deviable in an e Iri ct ro 3 1 at i c field, since Ktiuf- 
rtjann in his ca-efully carried out experiTnents obtained 
results which ivere in sucn extrenely good agreement 
v/ith t:-iecry. Bftsitjes^the d i saf r e e-ient of the -na';netic 
results .vith those obtained by other exper i'nen te r s , 
see".ed tc yhc'y th-^xt tr.e're .'/as ■:reBent Kcne p nenome na >vhi'jl 
v/ere affecting both alike. ^Iothinf has bee>". said thus 
far in these experiments concerning the effect of the 
seccndar-'- >'a3''s ivhi ch are produced 7/hen the 3 and V rays 
strike upon varr'ous substances. Tliit; effect vas froin the 
first concidered, and vas thourht tc be toe c"iall to 
a c c c u n t for the results obtained, b u t ^ a f t e r some f u r t '.1 e r 
exper i r.ent s , tho conclusion 'vas reached tiiat it played 
in all the experi-nents a lar^e role yxnd in sone cases 
theprincipalone. 

'^hen the R rays, cut down to a narrow pencil by 
neans of slits, v/ere alloved to pass through an open- 
in f in the bottom of the electroscope considerably 
v/ider than the supposed 'vidth of the nencil, it was 
found^on pi icing a narrow strip of lead over the opening 
in different positions to cut off only a portion of the 
p e ■: i n g at one t i ti e , t n a t the decrease in ionization 



13 



was the sa^^e for any part of t!ie opening. This sho'.vec" 

cZearly that the. rays coirinr throuf;h the opeinr itere ?:ot 

corfined to a narrow pencil as supposed but spread out 

into a diffuse, unifor^ily distributed beam. 

A photof^raphic plate placed over the opening siiowed 

on d evelopr".ent a broad, unj f or-^ily dense iTnaf:e instead 

of the sharp narrow one, which ought to be "lade by the 

3 rays alcne. This broader. in- of the pencil of the 

rays is unquestionably caused by the secondary radiation 

produced by the pri-nary 8 and y rays. If this secondary 

radiation was of the nature of yrays^then it wculd not be 

deflectal)le in a nap-netic or rI e ctro st :it J c field, and 

could con sequent I3; not affect the '^ ravs, but if on 

the other hand it vas of the nature of the primary ? rays, 

and therefore deflectable, great confusion would arise 

fro^ the different radiations. 

The secondary radiation produced by 8 -ind rays of 

radium has been the subject of i nvps ti ^^at i on by ''cClel- 

12 3 

land , Eve , and Kucera ,who found that in general it 

is of several kinds, both deflectable and n on- deflecta- 
ble in a magnetic field, and of different penetrating 
power. No definite knowledge was obtained of the velcc- 



1. Phil. 'af. 4Ur]'id 

2. Phil, "ag . tJhLC S'^o'^ 

3. .'Innalen der Physik. \*]oif 



14 



ities of the deflectable kind , and to this purpose the 
author decided to -lake a complete i n vo s t irat n on of t'-ie 
seco-idary rays. Before j'iving an account of this inves' 
tip;ation I would like to describe t ato experiraants on 
the 8 rays "lade by the pho to.c^r aphi c .-nethod. 



PHOTOGRAPHIC E XPSRIHE MTS. 

Ejep e r^3 m e_nt_ ^ . - The arr iinge'nent used in this is es- 

1 
sentially the sane as that used by Becquerel and is 

shown sketched in fig. V, Two netal plates a and b 
4.3 c Ts. in len,r;th \vere placed parallel to one another 
in a vertrJcal position 6 m-n apart, and insulated by 
'neans of ebonite. About 2 ens. belo/; the plates was 
placed the radiu?n, ccntainsd in a n-irrow creva?se in a 
block of lf"id. In the centre of the radium, -ind midv/ay 
bet'sreen the plates was fastened a sheet of "^ica c, \v;-!ic'i 
extended from the radiuT, up to the pho t o p;r aphi c plate e. 
This plate v/as v/ranped in a sheet of black paper , and then 
pl^jced Tn.-ide a lir^ht tight box containing a thin alumin- 
ium wnndow throu,q:h v/hich the rays could pass without 
"' u c h absorption. The distance between the top of t ii e 
netal plates and the photofraphic plate "fas 2.4 c-is. 

When the plates a and b are unchar'^ed there ourht to 
be obtained on the p -lO togr afthi c plate an imaj-.e cros:;ed 



1 . 1 c . c i t . 




F.gV. 



15 



in the centre by a nurruv/ band. On the other hand when 
th.e plates are charged to a hifj'.h potential if the rays 
are deflected to one side, the pho t c graphi c plate s^iould 
sho'.7 a broad shadow cast by the nica i-creen. In A and 
B, f:.?:. 6, are shown two photofraphs obtained by this 
method, A taken ".vithout an electric filed, ■■ ■' B v/ith a 
potential differe>Tce between the plates of 3000 volts, 
corresponding', to a field strength of 6000 volts per cm. 
Both photof.raphs appear p'^ec.isely alike and she?/ no indi- 
cation of any shadow on the plate. One side in both 
photographs appears darker than the other; this is on 
account of t^ie mica screen not beinj: plviced exactly in 
the middle of the radium, thus throwing ncre raTrs to 
one side than to the other. In C & D are shown two 
ph(-, + o^raphs taken with the screen pl;'ced exactly in the 
centre, C bein<^, v/ithout a field and D v/ith one; and both 
sides of the imape now appear equally (len^em These ph.o- 
to'-raphs were all taken with the radiun covered with a 
thin sheet of nica, so that no emanation could escape 
and affect tiie plate. Experiments viore also tried with 
the radiun uncovered, and the sane results were obtained 
as before. Radiii.m when dry and at ordinary t e^^perat ar e s 
does not give off verv -nuch emanation. 



n^M 



16 



Experiment II.- The arr anfj.e'-ent used in thic oxp eri.-r.ent , 

•xn.d illustrated in fig. 7, is essentially t.ie t;a-r,e as 

1 
that iiEod by Kaufinann in his work. T'./o brass plates, a 

and b, pliced parallel to one another inside a brass box 

A , \'iere i r. i; u 1 a t e d f r o n the sides by ''' e n n s of ebonite 

bushinf.s c and d. Beneath the ;ilates was ''as termed a small 

speck of radiura bro."iide, 'xnd above the plates a t'^ick 

ebonite screen •■vhich had a hole 0.5 mm cut in it, through 

which the rays could pass in a narrow pencil. At the 

top of tiie brass box vas pi •iced a pho to.rrraphi c plate 

wrapped in a sheet of black paper. The vhole apparatus 

was enclot,ed inside a 2^1ass vessel which could be exhausted 

to a high vacuum. /"- ^^ ^^^^^ ^^"^^3^ 

Exposures of one , two and four d a^r s v/ere made, but in 

A 

no case could any sharp image due to 3 rays be obtained 

on thie plate, the only effect being a darkening of the 
v/hole plate due to y and oedondary radiations. Hhen 
the radium was left uncovered the darkening of the v/ ole 
plate .'/as mucii greater, due to the emanation diffused 
throii^ho'i t \ ^-'^ ■: ?;sl . 

In another ar"angement a larr;er quantity of radium 
conta.-^ned in a lead cap.sule v/as pi .cec' outside the brass 
box, anr: ♦^.hp r.-\-'o allov'/ed to enter tnrough a small hole, 

1. loc. cit. 



/,v///////^//////j/j////f//^mA 




Fig^zir. 



and thence through an ebonite diaphrasra pLuced just 
ber. eath the brass plates a and b. 

This faflsd to give any better results than before; 
and all further attempts to repeat Kauf-'ann'n exper^nent 
•vere then a'bandoned. Proba^.ly irith better pho to." r aphi c 
Ekill in restrainins the darkening effect due to the 
rays I mij^ht have :-.ucceeded in obtaining a clear imacre 
of ";he p rays. The radi uni U£-.ed in thi. experinent •.vas sor.ie 
kindly loaned ine by Profestjor Rutnerford, and »vas as 
strong, if not stronger-, t.-ian that used by Kauf-:iann in his 
last experiments. 



SE CONP ARY RADIATION. 
The experimental ar^'angement ui^ed to study the 
-ecrndary radiation is shown diagr amat i cally in fig S. 
\bout 300 ;nilligranmes cf radium bror^.ide of about 30000 
activity 7/ as sealed in u very ti-in glass tube of 1.5 :;i!n 
dianetsr and about 5 cts. long. This tube v/as enclosed 
inside a lead box a, .-/hich had a ilit 5 c^is. long and 
1 '^:-i wide cut in one side, tnu -.vails of the lead box being 
of such a thickness that no ,3 rays could pass through. 
This box .'/as ce.'^iented to tv/o thick ebonite blocks b and c 
in such a nan-ner, that one edge of the i^lit coincided 



D 



^ Electroscope , 




FigMl. 



with a face of one of the blocks as indicated in the 
figure. ^ d^verrent bean of '^ - -- - t'-u^, f=-..r-ed fro-n 
the clit.ar.cl vas limited in svidth by the .valis cf t.-.e 
ebonite blocks. This apparatus v;as placed -O" thfcit the 
rays travelled in a horizontal direction. 

Directly above and purallt'l to the ebonite blocks 
v/as supported a thick screen A ,con str acted of cardboard 
and filled v/ith -ercury, and iiuving in tne centre a '^/ide 
rectangular opening throuGh ^/nich the radrut^ons could 
pass into a gold leaf slectroGCope placed above. The 
substances whi en were to be stL^died as sources of secon- 
dary radiation were pi iced beneath this opening in such a 
position that the f3 rays fell full upon them. The tnick 
nercury screen absorbed a large part of tne radiation; 
and althougn it introduced a snail a.ount of secondary 



radiation, this incretiee was r^ore 



than offset by the 



decrease of the rays. The ionizat:on in the electroscope 
due to the secondary radiation fron: below would under these 
conditions forn a -luch lar-er prop.-rtion of the .v-ole , 
tnan .v::en the full rays were present. 

iVhen tne radiator d is not present , the ionization 
in the electroscope is due to V rays and to secondary rays 



K 



produced by then. 

Tnen the radiator is placed in position this ionization 



19 



will be increased by that due to the secondary rays fron 
below. i-iy fixing rad'ators of different rnaterials in 
tne pcaition d, and pl^-cin" screens of varying absorbing 
power under the opening 3, a knov.'ledge of the relative 
penetratiing pov/er of the. secondary radiations from tne 
different radiators can be obtarned. "hen a t.aick screen 
is placed so as to cut off tne 1 rays, then the increase of 
ionization vjll be due to tne secondary rays caused by 
thefrays striking tie radiator d. 



Radiator - ^ir and -urruundinf Objects. 



Total Rate 
of Leak. 



3.C1 

6 .0^ 

2 .9-i 
Z .85 
,' .70 

3 .28 
3.29 



Hate of Leak 
due to Secon 
dary Rays. 



1.01 
0.4-2 
0.34 
.25 
.10 
.68 
.69 



Absorb- 
ing 'Ma- 
terial. 



j -t s h e e t s 
I paper 
; 8" •• 

16 " 

3-1: " 

5 " 




liUnab- 

sorbed 

Ray s . 



100 
41 
34 
25 
10 



Remarks . 



'lo rad : ator at d . 
Paper placed on 
top of "er- 
c u r y screen. 

Paper placed below 
screen placed over 
3 rays. 



20 



Radiator - Zinc. 



Total rate 
pf leak. 



10.20 
8.85 
7 .76 
6.21 
4 .7-t 
■i . 09 
3 .53 
3 .28 



Rate of leak 
due to r, econ- 



dary Rays . t e r .1 a 1_^ 



7.10 
5.7 5 

i . 66 

3 .11 

1.C4 

.99 

.4-3 

.18 



'absorb- 
ing "a- 



Paper 
2 " 

4 " 

8 " 
16 " 
24 ■' 
40 " 
60 



^Unab-" 
sor bed 
'"-■ ays. 

100 

81 

66 

44 

23 

14 

6 

2.5 



Re •^. ark s . 



In this set 
of readinp, s 
the absorbing 
layers of paper 
.vere placed 
directly over 
r ad i at or d . 



R ad i at or - Zinc . 



5.00 


1,90 


It 


100 


rays partly 


4.51 


1.41 


4 


II 


74 


screened by 24 


4.18 


1.08 


8 


II 


57 


sheets of 


3.80 


.70 


16 


II 


37 


paper 


Radiator - 


Zinc . 








3 .82 


0.72 


II 


100 


P rays screened 


3 .59 


.49 20 


II 


68 


by piece of 


3 .42 


.32 


36 


11 


44 


zinc . 


3.31 


.21 


86 


It 


29 


\ 



21 



Total Patej 

of leak . 

3.82 

3.30 
3 .2 k 



'•or re c ted I Absorb.! ng 

Leak . L ' 'i- "t o ria 1_. 

"6 



3.10 



Radiator 4- sheets of 
4.9 6 

4-. 18 

3 . 69 

3 .34 

3.21 



.20 
.14 

.00 



Paper. 
1.86 

1.08 

.59 

.24 

• 11 



i^adiator 8 sheets of 
5.29 



Paper 
2.19 



Padiator 16 sheets oi 
5.81 



paper 
2.71 



Padaator 28 sheets o 

6.4 5 

4.8 
4.13 
3 .57 
3 .29 
3 .23 



P 'ip e r 
3.35 

1.70 
1 ,03 

.47 

.19 

.13 



Radi-itor ^^lass 

7.52 

4.8 6 

Radiator Load 
11.36 

6.85 



4.4 2 
1.76 



3 .20 
3 .75 




ICO 





10 
32 





4 

8 

16 

32 

82 




8 





8 



^Ilnabsorbed 
Rays . 



100 

100 

70 





100 
58 
31 
13 

6 



100 



100 



100 

51 
31 
14 

6 

4 



100 
39 



100 
45 



Remarks ♦ _ __ 
Zinc screen over 

3 r ay s . 
2 7inc screens over 

^ r ay s . 
2 Zinc Gcreens over 

3 rays. 

radiator removed. 



Raddator Copper, 



Total Pate Corrected 

o^f L e aj: . I lieak . 

8.78" '" |~5.68 



^ad 2 at orlron . 
8 .69 

5.3 t 



5.59 
2.24 



A b s o r b i n r, 
■'aterial . 








8 



/' U n a ij s r b e d 

R av s . 



100 



100 
iO 



j-rom a study cf these results .76 see at once that, s -;b- 
stances wheii t; truck bv 3 rays eive out seconcary rays, 
■.vh3 ch differ anongst thenselves bcfn in quantity and 
penetrating po.ver. 

In o^'der to produce the maximum a lount of secondary 

rays the sibstancr, has to be of sufficient thickness to 

completely absorb all the ? rays which fall upon it. The 

amount of secondary radiation due to theVrays is only 

a very small quantity of tne total, provided the thickness 

of the radiator is only just sufficient to absorb all the 

P rays. 'Hhen only the ^.ost penetrating, rays are allo^ved 

to fall upon the radiator, the secondary radiations pro- 
sryu a/w. (KA^c\^A^c^ 

duced ire of u .ic-. -.ore penetrating nature, than -vhen all 
/\ 

the '^ rays are present. This is partly due to the fact 
that tne secondary rays due to tne hij^h velocity rays 
are -^ore penetrating, and also partly to the presence of a 
snail a-i.ount of se c end ary v' ray s cau:ed by the primary rays. 



\ 



23 



The denser a substance .is, the [^ r e a t e r -Mill be the 
a-rount of the secondarjr rays produced, -ind "he p;reater 
their penetrating power. Of tnoae substances exa-'ined, 
lead proved to be the most efficient, and also gave rajrs 
of the Tiost cenetratdng power, while paper .'/as the least. 
For the sake of comparnson I give in table II tne results 
of an absorption test on t -le primary S rays, (v/hich of 
course contained a certain a^iount of secondary rays), 
together v/ith the results obtained for the secondary ra- 
diation frcm zinc and paper. 

TABLE II. 



Layers ~i 


Prinary 


Secondary 


Secondary 




of Paper. 
_ 


B r ay s 

ibb' 


f romZinc 

"ibb'"' 


from Paper - 

ibb 





2 


82 


81 






4 


70 


66 


51 




8 


52 


44 


31 




16 


33 


23 


14 




24 


22 


14 






32 


15 




6 




4-}- 


9 .7 


5.8 






6 


5 .0 


2.5 


1 





24 



The penetratintT pov/er of the secc?Tdary rays fro"! zinc 
does not differ very ^.reatly from that of the pranarj' 
fl rays, especially for the f?rst few sheets uf paper. 
The penetrating pov/er of the secondary rays frorn lead 
is only slightly greater than th;it cf the rays from zinc. 

In fig. 9 are drawn several absorption curves, both 
for the primary 3 rays, and for the KecondarTr ra3/s. 
.'V represents that for the P primary rays, li that for tne 
secondary rays from zirc, C that for the second ar3'' fro"! 
paper, I) t^ie secncary from zinc when the pri-^ary R ravs 
have pastsed through 28 sheets of paper, anc": E that for 
the secondary from zinc when the primary S rays have 
passed through one shee' of zinc '''t is seen at once 
from thfcse curves that the radiiitions are not homo- 
geneous, but travel at differe-^t velocities. 

It is '.veil known that a purt of tne secondary rays 
are deviable in a magnetic field, and in the same di- 
rection as the 3 ra^'s would be. The magnetic deflections 
of the secondary rays from lead, and from paper, were 
tried h" t'-^e method illustrated in fig. 10. Tiie primary 
B rays from the radium enclosed in the lead box a strik- 
ing the radiator b, produced secondary rays which passed 
up into the el r c t ro scorje . Screens of lead c and d were 




n^.iK 



25 



so placed that the secondary rays frcn the radiator could 
juct touch the upper eAr'.f> E of the Tiercury e ere en. Kxper- 
iments wore perforr^ied vvit:'. both lead and paper as radia- 
tors, and in both cases it h'xs found, that the secondary 
rays produced .v/ere def]pcted tov»'ai'ds the ri.'^ht, v/iien a 
mannetic field was applied in such a direct?or. , that tne 
lines of fcce can be !-epresented ag goi nr into tne plnne 
of the paper. The results obtained in t.nic experi-nent are 
expressed in tne f o 1 1 o v : n " t a i) 1 e (III). 

T\BLE III. 
(Field' "s t7e ng t h 



1 Und e f 1 s c t e_d_ J' ay s] 



lead 


p ap e r 


ion 


100 


66 


58 


36 


6-i 


21 


28 


11 


li 


8 


10 





90 
180 
270 
380 
450 



Thsfje results show that the Keccndary radiations from 
both "letals and insulators consist for the T.ost part 
of negatively char?;ed particles. Those from insulators 
are -^vre easily deflected than those from the more dense 
metals, but the difference is net very pre at. The pro- 
portion of non-deviable rays in the secondary rays fron? 
paper is gr&atar tiian in that from zinc. 

TERTI^r.Y MYSj^ 
When the secondary radiation strikes upon objects 
there is produced a third type of radiation called the 
tertiary rays. Thir. radiation has been studied in the 



E/ecfroscope 



Merc api/ 



A / 



Screen. 



A. 



\y^ 



T^ L -' SP 




Radium 



F,g.T^ 



ze 



present investigation for -sl few substances. l';- o -ethod 
e-'iployod .vas precisel^^ the sane as that ured for the 
seconcary rays, with the exception that thR s-^al] ?^lass 
tube containing the radrura, instead of beinr placed in 
front cf the opening in the lead box, was "lOved to one 
side so that no (3 rays could emerge frorr the opening. 
Under these conditions the f^ rays will strike the lead 
walls of the lead box and -reduce secondary rays which 
will travel cut tlirnugh the opening. 

If :re nlace a radiator in the sane position as 
before, tnere will be produced i" it tertiary rays, 
which can pass up to the electroscope, anc cause an 
increase of ionization. Tne penetrating power of these 
rays was studied for lead, zinc, and copper radiators, 
and the results are sxpressed in the follov/ing table. 

TABLE IV. 



Layers of 




Tertiary ^ 


Paper 


Lead 


Zinc 





100 


100 


4 


59 46 


8 


35 


25 


16 


17 


10 


24 


6 


,i 




27 



A.S in the case of the secondary rays, lead proves to bo 
the most efficient radiator, and al&o gives out the 
greatest penetrating^ rays. The penetratinp po.ver of 
the tertdarjr rays is considerably lesf> than that of 
the secondary, that for lead in the former beiir only 
slightly/ greater than. for paper in th« latter. 

To find out tvhether th.e tertiary rays were ceviable 
in a mapnetic field, the arranjenent shown d iagr amat i cally 
in fig. 11, .'/as made use of. The rnercury screen A .vas 
placed so that one end -vas directly over the ends of the 
ebonite blocks a and b. The electroscope B was placed 
near to the edrie of the screen A, and had a v/indow c 
covered with tb.in foil cut in one side, so that any rays 
might enter without absorption. 

"I'aen the screen c was placed in position the tertiary 
rays produced could travel upv/ard and en«ter the electro- 
scope. '.:0W by placinr tv/o screens, d and e, in the posi- 
tions indicated in thf^ figure, the rays could be pre- 
vented from entering the electroscope, but a portion 
would still be able to travel up'vard. '.Vhen a magnetic 
field was applied in such a direction that th.e lines 
of force v/ere perepndicular, and going into the plane 
of the paper, the ionization in the electroscope v/as 
not appreciably altered, but when applied in the reverse 




Radi'i 



(SS 



SSf 






Fis-II 



28 



directicn there vas observed an increase in ioniza'ion. 
"oreover, when a screen was placed so as to cut off 
entirely the tertJary rudiatitn fro^i LpIoat, thi- effect 
was still observed but to a -^luch less de ree. These two 
^e^■ults indicated that thre was or e c en t ^ be si d e r: the 
tertiary radiation from below-a radiation which seemed 
to come from the -lercury near the /nndow of the electro- 
SCO e. This latter radiation is uidoubedly caused by 
the y rays when they emerre from the surface of the mer- 
cury, and is the same as that observed u- Kve nher\ tne )r 
rave were pirtly absorbed by a thick block- of lead. i3y 
placinp sheets of paper in front of tne window, it /as 
fo'ind that the penet ating pcver of this radiation was 
much less than that of the tertiary; t sheets of paper 
cut it down to 30^ , and It: sneets completely absorbed it. 

It >'/as also obi-evred that .viien the mapnetic field vas 
increased slowly from zero, a certain .-trength was 
reached at vhich the increase of ionization in the elec- 
troscope due to the tettiary rays from below just became 
noticeable. 'hen this hap'^e -.ed ^t he ravr from below were 
bent so that the extreme eC^re of tne beam just entered 
the windoiv. ''.noving three points on the circular path 
of the ra-i's the radius of curvature could at once be 
1 . loc . c i t . 



29 



calculated, and .vas found to be about 17 cie. Vhe 
strength of the r^aj^netic field .vas about 90 C . C- . o . lines, 
so that ve pet for the tertiary rays a value of H_fv = 1330 
approximately. These results shov^ that the tertiary rays 
are deviable in a marnetnc field in the same direction us 
the R anc secondary radiat:ion. They :iust therefore be 
ner.'^-ti ve ly charged particles travelling at apeede only 
a little lesii than the slo.vest p particles. 

'.".'hen the screen f is pl'iced in the position inciicated 
in the firfure, it .vas found that tae ionization in trie 
electroscope v/as increased. This ■vas found to be partly 
cue to the seccndar-"' rays produced v.-.en they rays strike 

the screen, and also partly caused by the tertiary 
rays froTi beloiv striking the screen, and producing a 
fourtn type of rays. 

That this latter ■'■adiation is present, can at once 
be shown by placing in front of the blocks a and b a 
screen, sufficient to cut off all the secondary rays, 
in which case the fourth rays are absent. This process 
'.vould probabljr go on for a large number of radiators, 
but after the third the radiation is too feeble to be 
measuT-ed accurately. Each type of radiation is of less 
penetrating power than the one v/hich produced it. 



30 



Velocity and ratio e for 'the primary 3 rays. 



It has just been shown th-tt the secondary 3 rays 
have nearly the sane penetrating pover ■xs the primary, 
and therefore, assjuning for the r^resent that they possess 
the same charge and mass, they "lUst travel at velccities 
only sl^phtly less. After passing through a certain 
thickness of absorbdnp; iniaterial, the lever limit for both 
types of rays ^ould be the sarne , and consequently the 
forv/ard edf^e of a deflected beam would consist of both 
primary and secondary rays of the same velocity, which 
■,7ere just able to pass through the absorbing layer and 
cause ionization. 

As the thickness of the absorbinp layer is increased 
the less penetratdnp; radiation would be -nore quickly 
absorbed, and at vsrv thick layers, the ed?,e of the 
deflected bean ,7ould consist almost entirely of the ".ore 
penetrating radiat'cn. 

If then by an^ method '.ve ca ■ find the forward edre 
of the deflected beam in both mapnetic and e 1 e c t ro s t ;.ti c 
fa elds, ve can at once calculate the velocity of those 
ra^'s, both primary and secondary, 7/hich are just able to 



Jl 



c aus eJ-cni Zfit i on after p. --is sin? thrcup-'o the absorbinp- 
layeTt The folHovinp method .vas t.en devised fcr this 
purpose anci proved successftl. It is sno.vn illusr.trated 
in fdg. 12. 

Two zinc plates, a and b, were supported in a 
vertica] direction, a^.d insulated fro.-n. one another by -neans 
of the ebonite blocks c and d. At the bottcn of these 
blocks //as fastened tne lead box containing the rlass 
tube of radium, tind f urni phed with a slit 1 ntiin in vidth 
thrcuph vhich the rays err.erred. A.t a short distance 
below the zinc plates there vas pi teed a lead diaphragm 
with another slit also 1 mm in .vidth, .vaich for-^ed with 
the opening below a narrow pencil of rays, ./aich travellee 
upward uetvveen the zinc plates. The distance between the 
two slits was such that the rays from the radiua just 
touched the top edjres of the plates. This apparatus 
was placed inside a pilass vesr-el A, which was clcsed 
at the top and iiottom with brass plates B and U . Ihroucrh 
the top plate B there .'/as cut a rectangular ope: in g 
1.5 cms in iriCth, and then covered .vith as thin a sheet 
of mica as would stand the pressure when the vessel .vas 
exhausted. The thickness of this mica window was about 
equivalent in absorbing power to 6 sheets of ordinary 
writing paper. The bottom plate C was pierced with three 



Electroscope- 




F'lg^IK 



holes, into which plass tubes were fitted, two of then 
f and g containing the connecting ffires K and 1., and the 
third H serving to connect the vessel to the pump. 

The whole appn-ratu<j v/as rendered aj r tipht by tne 
aid of sealinp --vax; afid it v/as founci^taut ;iixn an occa- 
snonil stroke of the pump the pressure could be -lain- 
tajned lc,7 enough to withstand a potential difference of 
10000 volts witnout a discaarge takin;^ place. 

'6v c o n n H c t i n g the .vires K a n r ' L to tne poles of the 
battery of lead accumulators, the zinc plates could be 
charged up to any desired difference of potential. In 
the meantime the nunber of the colls had been increased so 
that a naximun potential of 90C0 volts could be obtained. 

On top of the brass plate B v/as placed the mercury 
screen E, described in the previous pa<^es, which served 
to cut down in a large measure tne y rays. Tne opening 
in this screen was partly covered at the top by a brass 
plate E so placed that no P primary rays could enter the 
electroscope. The ionization in the electroscope would then 
be caused by V" , and secondary' ra-"s. 

The vessel was placed bet'/een the poles of a larre 
electromagnet, of such a size that the rays during their 
entire course la" in a uniforn field. 



■6'6 



When the primary rays strike the sides of tne slits 
in the lead d i aphrafrn-is , neconclary rayc -ire produced wiiich* 
travel ur>\/ard -.rith the prinar3' to the e 1 p c tro sco e . T.he 
pencil of rays at the electroscope is then -nade up of both 
primary and secondary radiation, but will be prevented from 
enterinF<ahe brass screen E. This nencil of ra^s '*ill, 
ho.'/ever, be confused by the presence of other secondary and 
tertiary rays coming from various points. This can be illus- 
trated by some photographs taken at different points alonp, 
the path of the rays. One taken 1 cm from the upper slit 
shows a narrow fuzzy imape, vhereas at 1 mm from the top of 
the zinc plates the image is sharp and the full •Yidth of the 
opening. \t the top of tne plate B the ircafe had again 
become indistinct, while at the top of the mercury screen 
it was of the full width of the opening and of uniform 
density. 

If the opening at the electroscope 'vas arranged 
symmetr - cal ] y with regard to the zinc plates, there was 
obfLeT-ved a decnase of ionization in the electroscope 
when the magnetic, or electrostatic fields were applied 
in either direction. The decrease in the case of the 
electrostatic field was about 25 per cent, with a strength 
of field of liOOO volts per centimeter. Thir, snows 
clearly that the rays are deflectable in an electric 
field, though the effect observed was onl'"' about one 



quarter as Kuch as n;ight be expected. 

■Vhen , hovever, the ar ranger.ent was the sa-e aa that 
described in fip, . 12, altopether different results vere 
obtanned. If tae plate a were charfred nefr,at a vely , the 
ionization increased gradually to a naxinum wit:-, increase 
of field, remained constant for a period, and tnen de- 
creased. If, on the otuer hand, the plate a is positive 
the ionization decreased at once. Tne reason for this 
can be explained in the follo^inr manner. 

If the plate a is charged negat i vely -the primary and 
secondary p rays will he deflected to the right^and enter 
the electroscope -thus causing an increase of ionization. 

This increase .'/ill continue until the rays have just 
reached the o p i j o s i t e side of the opening into the 
electroscope. ''!her\ this is the case //e can assume that 
those rays which after passing tnrough the; :» - c a o r b i r. g — lay o t 
can just affect ionization, are bent the most, since 
all rays of lower velocity, and hence penetrating yover 
cannot get t arc a gh . \ '> \o - 1 '■.y fiV - o The same phenomena 

exactly ,\rere observed \'tat^n a magnetic field was apolied. 
Consequently whfin the ^.aximum point is reached for both 
magnetic and el p ctr o s t at ic dfi f 1 cct ion , the value of the 
velocity of the L-lo./est ray, which can just get through 
the ajsorbing laj'er, can at once be calculated from tno 
values of the electrostatic and magnetic fields. V/hen 



^^ ^ 



35 



different thickn eases of absorbing layers .'/ere placed 
over t.ie openi^ig, the strength of fields necessary to 
produce the .-r. aximun ionization .vaa found to incr^-ase 
.vith increasing thickness of layer. T'r.ic is //hat we 
would expect if the rays are of all different veloc- 
ities, and cho 75,that v/hen the maxirau-n point is reaciied 
the least penetrating;; rays for each successive layer 
have all been bent through the sa 'stance. 

For the sake of illustration sone of taese results 
are expressed in the ac comp unyin<^. table (V). 



Through 


3 sheets paper 


\i4 sheets paper 


1.5 mms 


. glass 


r.PLVolH) 


/ia+e o/ Ucck K 


Pf6^vo(+6^ 


(ial€o±LenK 


mi^Qiti) 


(laieof^l^e^K. 





ll'l- .Osec. 





151.0 sec. 





154 sec . 


2700 


13 4.4: " 


3 400 


l!r4.2 " 


rOOO 


tl5 " 


3 000 


• 13 2.4 " 


3 6 00 


143 .4" 


5 6 00 


14 3 .4 " 


3 3 00 


131.G " 


3 9 00 


142.8 " 


58 00 


148.6 " 


3400 


131.2 " 


4100 


141.5 " 


6600 


148.4 " 


3 5 60 


131.0 •• 


43 00 


141.5 " 


68 00 


143.6 " 


38 00 


13 0.8 " 


C.O0O 


141.4 •• 






5 000 


13 0.6 " 










6000 


13 0.6 " 











tax. 3500 Volts - 



4100 volts. 



6000 volts. 



In this method v/e do not kno// ho// far eacii ray is bent^since 
we do not k n o v/ its first position, and therefore cannot 



iib 



Obtain values of jViV, and MV , ''Ut since the deflection is 

s'liall compared to t'ne len.gth of tue path, we can assume wit^ioat. 
any n;reat error, t:.it^ for a maximum, this is thw sa^ie for both 
nac?netic and electric deflection. 3y comparing the e.ljctric 
and magnetic forces on the particle v/e can a,t once esti';u.te 
its velocitj^. If d is the distance travelled 03' the ra;' in 
the uniform magnetic field H, 1 the lengtli of the zinc plates, 
h the distance from top of plntes to olsctroscope, X the 
strength of e 1 1- c t r i c field, the, v e 1 c i t j'- V is g i v e ^1 by, 



V 



Hd 



j- 



In this experiment, d = l?.*^' cris. 1 = 8.4 cis , h 
the distance apart of the char.t^ed plates was 6.2 
fore , 



J.J c 



na 



mms , there- 



As an example take the results for an absorbing layer of 

11 
6 sheets of paper; here X. = 3500 = 5.7 x 10 C . C- . S . and 

0.C2 
K = 13.5 C.O.S. lines, and therefore ve obtain, 

11 10 

V = 0.5 63 X 5.7 X 10 = 2.37 x 10 cms / -ec. 
13 .5 

In order to obtain values for iS_, it is necessary to know 

either Tm . or V\V, for the different ravs. Values of TnV 

6 e e 

were obtained by the folio./ JnH method. 



37 



The lead dox co 't -ii nine; tht; radian tube vas fastened to 
the ebonite blocks as before, but tne di. stance between 
these narro.ved to 2 n.'ns , and the upper lead disphragm 
removed. This ar ''•i.np.enent allo.'/ed a broader pencil of rays 
than in the previouL- experiment to pass upward to the 
electroscope. Tv/o zinc plates ii cms in height ^rere fas- 
tsned to t;ie ebonite blocks in a vertical directior: and 
so arranged that one edge of the pencil of rays could just 
touch the top of tne one of tne plates. The effect of this 
upper plate ivas then to define siiarply a pencil of both pri- 
marjf and secondary rays. This arrangement ^as then sur- 
rounded bv a magnetic screen of soft* stieet iron v/hich ex- 
tended up to the top of tne z«nc plates, and kept the rays 
during theJr passage bet.veen the plates from tha action 
of the Magnetic field. The glass vessel was dispensed v/itn 
anci thfi pxneriinent perfornied at at:r.o spheric pressure, sheets 
of paper equivalent in absorptive po.ver to the "ica v/indo.v 
of the •previous experiment being interpcsuul in tne path of 
the ra^'s. The opening at the. el ac tro scope , 1 cm in v/idth 
was arranged as in t)ie other experiment so that no rays 
of this pencil could enter ':he electroscope. 

'Vnen a marnetic fielf' v/as :inolied in the proper di- 
rection t:.e ionization in the « 1 i-ctro s cope gradually in- 



;i8 



creastid to a •naxi.'tura as the, strenptn of the fielc^ '.ras irr 



c r e a 15 e d 



1 n c e z 



h? rays are only under the action of tns 



nai'netac field during their passage fron the top of the zinc 
plates to the electroscope v;e can as g u^ie t .lat ^ '.vhen the naxi- 
mura po^nt is readied, tne leaat penetratinp rays have been 
deflected over the distance represented by the '.'fidtn of tae 
opening. By placinp, in the path of tne rays suitable thick- 
nesses of absorbing 'TiaterDal the value of JJlVfor the sane 

e 

rays as were ob.served in the previouL^ experiment could be 
ascertained. 

These values 'vere calculated fron the f ol lo .'/in? for- 
nula , " ( See J. J. Thomson's, Pischarf^e of Electricity 
through Gases.,, pa r, e 92. 

//hereO= the distance taroafh ./hich the rays are bent, and 
H the value of tne "lapnetic field at d:^fforent porlnts along 
the Tath of t n - ravs. The value of )Tiy obtained bj' t.'iis 

^ " 3 ~e 

;-ethod was 1.57 x 10 for no absorber, whereas, for 1.2 '^.m of 

3 

zinc it 7/as 5 x 10 ; for C siieets of paper corresponding to 

2 

the "^.ica v/indow tie value ".vas 1.87 x 10 . 

In the forr.er experi"ient in the uniform field the value .-tf*^"^ 
of yyW- n (^ , and substituting the • ; ?»< > ■». « valuer of IfYW/^ .'/e ret 
for the distance thro'irh vhich the rays .vers bent 1.04 cis. 
Knov^ing this value of u all the remaining values can at once 
be calculated, and the complete results are sacvn in the 



39 



follov/inr; table (VI). 

T.\3LE VI. 




6 of paper 
10 
14 
18 
22 
3 " 



X(nv^>) 



1 



11 



5.7 xlO 
6.1 " 

6 .G " 
7.2 

7 .7 

8 ..i 



1 . 5rnm g^ ass) 9 . 6 



13 .5 
l-t.3 
15.1 
16.2 
17 .0 
17 .9 
20.0 






•2^ 



.3 coppef 
0.4 zinc 

.8 " 
1.2 " 



11.0 
li.O 



22.2 



13 



4.4 xlO 
4.76 
5.15 
5.62 
6.01 
6 . kl 
•1 . 49 
8 .58 






3 



27 



.2 0.0.9 2 



1.57x10 
1.87 
1.98 
2 .10 
2 .25 

2 .3 6 
2.49 
2.78 

3 .09 
3.7 9 
4.6 
5 .00 



'^Cm^j, 



Uc 



2 . 2 ; e s -t . ) 

10 
2-37x10 

2.40 

2.4 5 

2 .49 

2. 54 

2. CO 

2 .09 

2.7 7 

2.88 

2 . 9 5(e E t i - 

2.97 ' 



m 



1.40 

1.27 xlO 

1.21 

1.17 

1.10 

1.07 

1.04 

.96 

.90 

.76 

.64 • 

.59 * 



i 



-\s has alreadv been exnla? n ed ^tne x'alues f^iveti in the above 
table .represent those for both the primary and secondarjf par- 
tides 'Vh:' ch are j'.'nt able to penetrate thro'uph a certain 
absorbing layer and still cause ionization; the highest 
values of the velocity are tncce for tr.e !3 particles alone, 
since nearly all tne secondarj' p'irt:cles are absorbed in about 



• These estimated values were extrapolated fron the curve 
showing the relation between the velocity and >nV. 



40 



35 sheets of paper. The values of the velocity for th.e par- 
ticles thro'^fTh 0,8 and 1.2 mm of zinc could not be ob- 
tained fo"* the reason th;t tne linit of the available) dif- 
fsrenco of potential nad been reached. The valuer of ihWfor 

e 

th?se, ho '/ever, show that the apparent -nass of the parti- 
cles ir increasing rapidly as the velocity of lif^ht is 
approached. The In.ver liTiit of the ^ rays camot be stated 

■vith anir certainty but it i c probably greater than 2.i x 
10 " 

10 cms per sec. T'ae *? rays in a]l the oxneri-ents had 

fnrst of all to pass- thT'oagh the thin glass walls of 

the tube, v/h:5 ch would probably absorb about as "luch as the 

n i c a w i n d o Af . 

The results f.iven in the above table apree vev' veil 

1 
with those obtained by ''auf-^ann in hi r later experi- 

■"ents, usinp; an entirely different method, and shov beyond 
doubt that the p particles from radium travel with speeds 
approachin,^ that of ]ight, nn6 further that their apparent 
mass does increase with the speed. 

In Kaufr^.ann's experiment secondary radiations must have 
been present in quantities quit© comparable with the prim- 
ary, and consequently any point chosen on his curved pho- 
tographic traces would represent not alone the primary par- 
ticle, but -^Igo some secondary particles v/hich happened to 
arrive at the sam.e point. If tr)e pri'iary and secondary 
1 . lo c . cit . 



il 



particles differed i 'o velocity there -njrht p...«ibly be 
sor^e ,^dff:caty in .st5-natin? tn. radii of curvature for 
the different ravs. He h.. cmpared his results ^i th 
those calculated fror. the theoretrca] formulae of Vora- 
ham, and fines a very close agreement, thus giving con- 
siderable evidence to tne view that the -.ss of the elec- 
tron is entirely electrical in orison, and increa.es as 
the speed apnroaches tp.at of liR^nt. The result of the 
present in vost i ~at i on also see--,s tc l.ad to the sa:^.e 
conclusion. 'Ve ^ust, no .ever . re-nenber that the confirna- 
tion of tni. tneorv is only over a short ran^e w;>ere tne 
increase of the aonarent -^ass is not very -reat, and 
vhere any F,et of values niPht accidently agree very 
closely v;ith the theoretical. It is not until the 
speed has. for all exparimeatal purposes, practically 
reached that of lip;ht that tnere is any ^reat increase 
of tne apparent mass, and consequently any conf i rn^.at ion of 
the theorv over a long range is entirely beyond exper- 
i-.ental nieans. "'oreover the a.-sumptions -ade in the 
deviation of tn.- theoretical forniulae, and also in the 
for-nulae used to calculate tne velocities and ratio e^ 
from the experimental data, are many and some'Vhat grea^. 
It is assumed that t ,« same laws of electric and magnetic 



42 

force apply equally well as very hiz'n speeds as at com- 
paratively low, somethinfr of .vh: eh wo have no a priori 
knowledge. ^ diver "ence of either, or both, of these laws 
at h5(^h speeds could -iccount for the ax^ er i-nent al fxcts 

observed . 

Hovevor considering; al] sources of error the re- 
sults of Kauf raann , together with those of the author 
lend great weij^ht to ths view that the '"aso of the 
electron ic electrical in origin, and increases with 
the speed . 



Velocity and ratio ^ for the secondary 3 rays 

"7n 



It has !)een assuned in the previous sections that 
the velocity of the seccnOary rays was only slightly 
less than the primary, and also that they carried the 
sane chars-e and had approximately equal Trasses. That 
these facts are true was proved by the follov;:ng set 
of experiments. 

The general arrangement of the experiments vas the 
same as that used in the case of the primary rays, and 
the same drawings and general description will suffice 
here. Thn tube of radium, instead of being placed under- 
neath the slit in the lead box, .vas shifted to one side 



43 



so that no primary raj's coulri emerge fron the box. The 
lead box was fastened to the ebonite blocks so that the 
slit .'/as near the rdpht hand block, and net in the ".iddle 
as v/as the case vitn the priTiir;' rays. The upper lead 
diaphragm :ra.B re'.cved and in its stead was fixed a strip 
of lead , which covered one t.aird of tie opeiinF belA'een 
the blocks. T!ie secondary rays on energinp: fro-n t.ie slit 
in t \e lead box could strike full upon tne left hand 
zinc plate ^but were prevented by this strip of lead fron 
falling upon the right hand plate. The rest of the ar- 
ranc^ement vas p'-ec-'sely the sa-ie as for tae primary rays, 
the opening at the electroscope being arranged so that 
no secondary rays from the lead box could enter. 

The secondar''^ rays when they strike the left-hand 
plate -,and also the edge of tlie lead .trip produce ter- 
tiary rays which travel up vith the secondary rays. \ 
great part of those will be absorbed by the rr,ic.a window 
but so-ne will get through and cause ionization in the 
electroscope. Tnere U. also a s'nall ar^cunt of secondary 
rays produced by the rays striking the various parts of 
the apparatus; these, however, do not affect the results 
since the- cone fror. all different parts of the vessel, 
and are therefore deflected verv unequally. 



•tl: 



When thtt elactric or -agnetic fiolcls vere applied in 
the sa-^e directions; as in the case of the primary ravs 
the sane phenonena were observed; a fradual 3r,crease of 
ionization to a maxinum //ith increasing fields, in one 



dnrectfon, -xne i decrease at on 



ce wit!! -Vl.e field an th 



other. The sa'^e abgcrb5np laj'ers were used in this case 
as in that of the prf^-nary rays. It vas fuund that no 
increase of denization above 30 layers of paper could be 
Ob erved, that thickness being sufficient to alr.ogt 
completely absorb the secondary rays. These results 
confirm the idea that tie secondary raye have a less 
penetrating character than the primary, and travel at 
lever cT.-'^.nds. 

Tn order tc pstin^ate how far the ray£.= rere bent in 
tne electr^-c and magnetic fields the same metliod .vas used 
as for the primary rays. Al ;! that ./as necessary to do 'Has 
to shift the tubo of rad-:an from beneath the slit in the 
lead box tc one aide so that no primary rays could get 
out. The soft .iron .ecreen v/as placed ,0 that the rays 
■rere shielded from the influence of the field until they 
had passed the top of th. zone plate. The distance from 
the top of the zinc plate to the electroscope //as less 



than in the case of t 



he primary rays, but tie ffidth of 



the opening in the electroscope the same. The value f >Tff 

e 



1-5 



3 
for r. c absorbing layer v/as fo and to be 1.56 x 10 ^ and 

for an a b sorb ring layer of 6 sheets of paper v/as 1.85 x 10 . 

These values a.re about the sa-ne as the c o t espc nci mg ones 

found for the priniary radiation, and she* that the lo;/8r 

limits :r ^'-.e latter case were those of the secondary 

rays. The upper limit for the secondary rays by this 

lethod .'/as also thp. gar-.e as by the otner method, viz., 

3 1 ay e r s of paper. 

r u b s t i t 'u t : n f^ t h « s e values of JTW in the; results 

e 

obtained by the fi»"st method v/e obtain 1.29 ens as the 
distance throur^h .yhTCh the ""ay ■ were deflected. 

In thic; experiment, 1 = 8 .-i: cms, h = 5.5 cttib , and 
d = 17,3 cris, :^r\6 therefore, 

In the. ac coripanying table(VIT} are expressed the final 
results obtained for the secondary rays. 

TABLE VII. 



\bsorbi ng 


"' ^ 




mY \ 


1 

V cirs/ sec 


.^ 


La;;er . 


X(:nax) 


H (nax) 


e ' 


m 








3 









+ 

11 


- 


1.56x10 


10 


7 


C paper 


6 .9x10 


If, 


1.85 


2.35x10 


1.27x10 


14 " 


7.5 " 


17 


1.97 


2.10 
2.50 ■' 


1.21 " 


2 2 " 


8.5 


18.5 


2.16 


1.16 " 


3 


9 . 6 •• 


30.:: 


? .36 ; 


2.58 " 


1.03 



46 



It will bei seen at cnce fri.m tnis table that the values 
of t'le velocity and ratio ^_ for the secondarv ravs are 

m 

in t'ood apreernent with those obtained for the primar'/. 
"ince the exr>eri-^ents on the secondary radiut.ions fru'n 
different substances, described earlier in this paper, 
showed th-it they were ?.ll deflected in a magnetic field, 
and since further that the penetrating power cf the rays 
vfrere not ,-reatly different, we can conclude that both 
metals and dielectrics J'ive off when struck by rays, 
negatively char-eo p^trticles .fi^h velocities, ;\r\c ratio 
( thp san.e as these for the less i^enetratinp S ravs. 

m 

■-.s to the origin of tnese secondary and tertiary 
radi at i^'ons , twc possible explanations can be given. They 
Tirht be the pri-:ary B p-irticles reflected back fro"i the 
"lolecules of the bonbarded substance. The ether and 
-luch more prob-i'De vie>v is that, the secondary radia- 
tions are pruduced Jfhen ine pri-nary 8 ritys, striking the 
r.toms of the substance, cause them to give off one cr 
nore of the electrons of //hich they are co-nposed, v/ith 
sufficient velocity to escape fr^m. the substance. The 
longer the path, and the greater the '^.umber of atoms 
which a particle encounters before it is absorbed, 
the greater ffil!! be the a-^. unt of thu secondary radiation 
produced. The nature and a'lount of the secondary radia- 



17 



tipne doMthe>iatiireoft'i'-atfc'". of 

♦'. n production of 

socontiar; tertiary rud ' is t .en . inilar in rna'r; 

reelect 8 tr. fl action of P rays by the radio^ictive 

i ul • '■ • • ■ '• * " ( " i - -IS f ttT as 

*e '-.•oti ^ ro n ♦ n-' Hi.u •• for"ipr JV is tiue to external 

agents. 

It *jll pern.'ips Lie instructive * ' e f ly sun.iiar- 

ize 'rxfiTo the main facts brourht out i- iv- 

\08tif-it3cn. 

The d5fficilty exp er n en ced at first in ootai -n 

L'l '^ctrc a t 'it i c defl ct itn of * le "^ riyt c^m to be 

secr.cary anc te'^tiary r ad J it i o n l. • 

''I'.e-i til is disturbinp, ictjicn had been t itec by 

f M r -,-<*-, f' Q •ion . ^ * . c i t y , -and 

'■ A t i o ^ , ./ e r e o u t a i n e c c s e 1 y * i t h t h t s e 

frund by ''aufmann usinr an entirely different "lothod. 



_ (» 1" •*(>•( ^ H r II'" 
a '^ e produced s .a- p r i r; 

inz rate'"?al, <-re conpticed of 
rZ r z t r ■'.".'{' 1 1 i :' 



,or-.,r-- TH'"" +'fns, y/hich 

s t,trike -pon an absorb" 
ively charred pxrti- 

t? :: nnnrl'- f? T •■ "! tc '-.it . <■ the 



18 



rays t ne-ise Ives , and hivinj^ the La"ne r-itio jS^ for corre- 
spondinp velocities. The ;: e c one' ar ■' vays t he" ce 1 ve s ^v/hen 
jncr'dent upon a sub stance «prc d u c e tertiary r ay 3 , vTh5ch are 
of slightly lesf; penetratinp, c hrir i^c t er , 'ire deflectable 
in a •naf.netic fi^ld in the sa-ie di'-ectnon us the secondary 
ai(i pr.-:~i>.y « rays, and are probably of the same nature 
as these. 

The values of _^ obtained for both the ornmary -xnd 
seconcar" n rays shoived, that t^ie mi^-'i ^r e n t "^'iss of tne 
part:'cles increased as that speed api'roacnsd the velocity 
of 1 i f h t . 

Taking f o - <-»-Hnted that the asf;umptions involved in 
t h ? c a 1 c u 1 a t :> o n s of the v e 1 (> c .i t y , "1 n d ^ , are correct, 

nv 

•ny •results together .vita those of "aufmann fur-iish evi- 
dence in favour of the view that tne maci. of the el;=ctron 
is entirely electrjcal in nature. 

In conclusion I vish to express my tincere thanks to 
^rofessor \?^!es for r.is kindly interest, valuable t.ug- 
festJons, and for the facilDties -.V'lich he Placed at '^,y 
comniand during the pronress of this i nve sti !-at i on . 



Johns Hopkins 'University, 

Balt-imore , "d . 
''arch, 19 PC.